论文标题

非线性相空间填充极化晶格的微观理论

Microscopic theory of nonlinear phase space filling in polaritonic lattices

论文作者

Song, Kok Wee, Chiavazzo, Salvatore, Kyriienko, Oleksandr

论文摘要

我们为在强耦合的二维极化晶格中开发了一个完全的显微镜理论,用于非线性相空间填充(NPSF)。在极化实验(NPSF的理论描述)中,无处不在,仍然仅限于扰动治疗和均匀样品。在这项研究中,我们超越了现有的理论描述,并发现了NPSF至关重要的光学响应的​​广泛范围。在研究非口号,合作光 - 偶联和库仑封锁的量子效应时,我们揭示了由于相空间填充而观察到非线性狂犬分裂淬火的几个制度。与先前的研究不同,我们将非线性的Rabi频率一直缩放到饱和极限,并表明晶格电位的存在会导致定性不同的非线性。我们专注于NPSF的三个制度:1)平面; 2)骨折;和3)超定位。在平面饱和度中,狂犬病频率随激子密度的函数呈指数降低。对于骨折的情况,激子形成一个晶格,其位点超过激子大小,我们发现晶格低职业的快速NPSF。随着培养基完全饱和,NPSF之后是较慢的NPSF。这种行为在库仑(或rydberg)阻塞的情况下特别明显,其中快速和缓慢的NPSF区域取决于排斥力的强度。对于超定位的NPSF,我们观察到两级系统收集的典型平方根饱和度。我们的发现可以帮助描述最近在过渡金属二分法的异叶剂中强烈非线性的观察结果,其中moir {é}晶格自然出现[自然\ textbf {591},61(2021)]。该理论还开辟了工程的前景,具有带有图案样品的极化晶格的强烈非线性响应,将北极星驱动到量子状态。

We develop a full microscopic theory for a nonlinear phase space filling (NPSF) in strongly coupled two-dimensional polaritonic lattices. Ubiquitous in polaritonic experiments, the theoretical description of NPSF, remains limited to perturbative treatment and homogeneous samples. In this study, we go beyond the existing theoretical description and discover the broad scope of regimes where NPSF crucially modifies the optical response. Studying the quantum effects of non-bosonicity, cooperative light-matter coupling, and Coulomb blockade, we reveal several regimes for observing the nonlinear Rabi splitting quench due to the phase space filling. Unlike prior studies, we derive nonlinear Rabi frequency scaling all the way to the saturation limit and show that the presence of a lattice potential leads to qualitatively distinct nonlinearity. We concentrate on three regimes of NPSF: 1) planar; 2) fractured; and 3) ultralocalized. In planar saturation, the Rabi frequency decreases exponentially as a function of exciton density. For the fractured case, where excitons form a lattice with sites exceeding the exciton size, we discover fast NPSF at low occupation in the lattice. This is followed by slower NPSF as the medium becomes fully saturated. This behavior is particularly pronounced in the presence of Coulomb (or Rydberg) blockade, where regions of fast and slow NPSF depend on the strength of repulsion. For the ultralocalized NPSF, we observe the square-root saturation typical to the collection of two-level systems. Our findings can help describing recent observations of strong nonlinearity in heterobilayers of transition metal dichalcogenides where Moir{é} lattices emerge naturally [Nature \textbf{591}, 61 (2021)]. The theory also opens the prospects for engineering strongly nonlinear responses of polaritonic lattices with patterned samples, driving polaritonics into the quantum regime.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源