论文标题

氦保留在干净W(110)中的通量依赖性:自我捕获的实验证据

Flux dependence of helium retention in clean W(110): Experimental evidence for He self-trapping

论文作者

Dunand, A., Minissale, M., Angot, T., Bisson, R.

论文摘要

在钨(W)中保留氦气是融合反应堆的关注点,因为它可能不利于面向组件的性能并影响融合燃料平衡的等离子体。他没有溶于W,它倾向于在先前存在的缺陷(空位,晶界)上结合,但从理论上讲,它也可以通过排放空位/自我解释W对元素的空位/自我解答W对构成母鸡的内在群体的自由度来进行自我陷阱(在非释放的空位上固定)。在本研究中,我们准备了一个带有干净表面的纯单晶W(110)样品,以证明在300 k的样品温度下,He在W中的自我捕获,并且以2.0x10 $^{21} $ He $^+$。$^+$。m $。m $^{ - 2} $的恒定通量。以130 eV的$^+$动能为0.3x10 $^{17} $ he $^+$。M$^{ - 2} $。S$。S$^{ - 1} $,我们只观察到一个小的He He Uneptight peakemption Peak在600 K以下,将ION FLUX升至0.7x10 $^17} $^{17} $^{17} $ he $^+$。m $^{ - 2} $。s $^{ - 1} $,我们观察到了在950 K和1700 K处的两个解吸峰突然出现。对于这项工作中最高的通量,5.0x10 $^{17} $ HE $^+$^+$。$。观察到1900 K。这些他解吸峰的温度位置与密度功能理论文献一致,并指出一次自我捕获的发生,一旦发生0.7x10 $^{17} $ he $^+$。$^+$。m $^{ - 2} $。S$^{ - 1} $ flux在300 k中实现了300 k的flux $ flux $ flux $ flux $ 5.0x10 $ a。 He $^+$。M$^{ - 2} $。s $^{ - 1} $。当前的结果应该用于限制HE保留的发展,并基于从头量数量起泡增长模型。

Helium (He) retention in tungsten (W) is a concern in fusion reactors since it could be detrimental to plasma facing components performance and influence the fusion fuel balance. He being not soluble in W, it tends to agglomerate on preexisting defects (vacancy, grain boundary), but it could in theory also self-trap (be immobilized on a non-preexisting vacancy) through the emission of a vacancy/self-interstitial W pair in the vicinity of a Hen interstitial cluster. In the present study, we prepared a pure single crystal W(110) sample with a clean surface in order to evidence the self-trapping of He in the W bulk at a sample temperature of 300 K and for a constant fluence of 2.0x10$^{21}$ He$^+$.m$^{-2}$. At a He$^+$ kinetic energy of 130 eV and a flux of 0.3x10$^{17}$ He$^+$.m$^{-2}$.s$^{-1}$, we only observed a small He desorption peak below 600 K. Rising the ion flux to 0.7x10$^{17}$ He$^+$.m$^{-2}$.s$^{-1}$, we observed the sudden appearance of two desorption peaks at 950 K and 1700 K. For the highest flux studied in this work, 5.0x10$^{17}$ He$^+$.m$^{-2}$.s$^{-1}$, an additional desorption peak at 1800 K and a desorption shoulder at 1900 K are observed. The temperature position of these He desorption peaks are consistent with the density functional theory literature and points to the occurrence of self-trapping once the 0.7x10$^{17}$ He$^+$.m$^{-2}$.s$^{-1}$ flux is attained at 300 K and to the possible realization of trap-mutation for the flux of 5.0x10$^{17}$ He$^+$.m$^{-2}$.s$^{-1}$. The present set of results should be used to constrain the development of He retention and He bubbles growth models based on ab initio quantities.

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