论文标题

纳米材料中局部和非局部冲击波的共存

Coexistence of local and nonlocal shock waves in nanomaterials

论文作者

Gianani, Ilaria, Gentilini, Silvia, Venditti, Iole, Battocchio, Chiara, Ghofraniha, Neda, Barbieri, Marco

论文摘要

高性能的纳米材料对于先进的光子技术(如传感,激光,成像,数据存储,加工以及医疗和生物应用)至关重要。金属纳米颗粒起着关键作用,因为局部表面等离子共振增强了宿主材料的线性和非线性光学特性,从而增加了应用的范围。改进的光学响应导致了富集且在很大程度上未开发的现象学。在目前的工作中,我们通过用脉冲激光束的金纳米棒的水性悬浮液来显示出两种色散冲击波的形成和相互作用。通过分析在色散材料中正规化冲击阵线的特征性孔,我们能够区分不同起源的分散冲击波,即电子和热的,首先共存,然后相互作用,然后相互作用以形成同等强度的双面前端。观察到的情景与现有文献一致,该文献报告了对包含金纳米颗粒的材料的非线性折射率的电子和热贡献。尽管对报告结果的全面理解值得分析描述,但他们已经为使用含有金属纳米颗粒的材料作为研究基本极端非线性现象的平台铺平了道路,并开发了用于感应和控制的新颖解决方案。

High-performing nanomaterials are paramount for advanced photonic technologies, like sensing, lasing, imaging, data storage, processing, and medical and biological applications. Metal nanoparticles play a key role, because the localized surface plasmonic resonances enhance the linear and nonlinear optical properties of hosting materials, thus increasing the range of applications. The improved optical response results in an enriched and largely unexplored phenomenology. In the present work, we show the formation and interaction of two dispersive shock waves emerging by illuminating an aqueous suspension of gold nanorods with a pulsed laser beam. By analyzing the characteristic undular bores that regularize a shock front in a dispersive material, we were able to distinguish dispersive shock waves of different origins, i.e., electronic and thermal, first coexisting and then interacting to form a double front of equal intensity. The observed scenario agrees with existing literature reporting an electronic and thermal contribution to the nonlinear refractive index of material containing gold nanoparticles. Although a full comprehension of the reported results deserves an analytical description, they already pave the way to using materials containing metal nanoparticles as a platform for studying fundamental extreme nonlinear phenomena and developing novel solutions for sensing and control.

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