论文标题

原子上薄的范德华抗铁磁铁FEPS3中的巨型磁各向异性

Giant magnetic anisotropy in the atomically thin van der Waals antiferromagnet FePS3

论文作者

Lee, Youjin, Son, Suhan, Kim, Chaebin, Kang, Soonmin, Shen, Junying, Kenzelmann, Michel, Delley, Bernard, Savchenko, Tatiana, Parchenko, Sergii, Na, Woongki, Choi, Ki-Young, Kim, Wondong, Cheong, Hyeonsik, Derlet, Peter M., Kleibert, Armin, Park, Je-Geun

论文摘要

范德华(Van der Waals)(VDW)磁铁是调整具有巨大潜在旋转物应用潜力的二维(2D)磁性的理想平台,并经过深入研究。但是,对于这些抗磁磁系统中磁性的微观起源知之甚少。我们使用X射线光发射电子显微镜来解决VDW抗铁磁铁FEPS3的电子和磁性,并向单层。我们的实验表明,巨大的平面外磁各向异性为每一个fe离子22 meV,并伴随着未淬灭的磁轨道矩。此外,我们的计算表明,FEPS3中的伊斯丁磁性是Fe 3D电子系统的自旋轨道纠缠的可见表现。

Van der Waals (vdW) magnets are an ideal platform for tailoring two-dimensional (2D) magnetism with immense potential for spintronics applications and are intensively investigated. However, little is known about the microscopic origin of magnetic order in these antiferromagnetic systems. We used X-ray photoemission electron microscopy to address the electronic and magnetic properties of the vdW antiferromagnet FePS3 down to the monolayer. Our experiments reveal a giant out-of-plane magnetic anisotropy of 22 meV per Fe ion, accompanied by unquenched magnetic orbital moments. Moreover, our calculations suggest that the Ising magnetism in FePS3 is a visible manifestation of spin-orbit entanglement of the Fe 3d electron system.

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