论文标题

石墨烯中应变诱导的Landau水平的可视化 - 黑色磷异质结构

Visualization of Strain-Induced Landau Levels in a Graphene - Black Phosphorus Heterostructure

论文作者

Vu, Thi-Hai-Yen, Lyu, Pin, Jo, Na Hyun, Trang, Chi Xuan, Li, Qile, Bostwick, Aaron, Jozwiak, Chris, Rotenberg, Eli, Lu, Jiong, Fuhrer, Michael S., Edmonds, Mark T.

论文摘要

应变诱导的伪磁场提供了实现石墨烯中零磁场量子大厅效应的可能性,可能直至室温,这代表了无损电荷运输应用的有希望的途径。石墨烯上的应变工程是通过底物上的随机纳米泡或人工纳米结构来实现的,但是高度局部和不均匀的假磁场可能会使电子结构的光谱探针变得困难。异质结构工程提供了一种替代方法:通过将石墨烯堆叠在另一种范德华(Van der Waals)材料的顶部,具有大晶格不匹配,并以所需的扭转角度叠加,可以在整个异质结构中均匀地产生大型应变诱导的伪磁场。在这里,我们报告使用纳米角度分辨光发射光谱(纳米弧)来探测石墨烯/黑色磷异质结构(g/bp)的电子带结构。通过直接测量石墨烯和黑色磷的Iso-Energy轮廓,我们确定了异质结构中20度的扭角。费米水平附近石墨烯带的高分辨率纳米孔揭示了位于狄拉克锥体内的扁平带的出现。平谱带的间距与石墨烯中的Landau水平形成一致,并且对应于11.36 T的伪场。我们的工作为研究2D材料和异质结构中的应变引起的量子霍尔阶段提供了一种新的方法。

Strain-induced pseudo magnetic fields offer the possibility of realizing zero magnetic field Quantum Hall effect in graphene, possibly up to room temperature, representing a promising avenue for lossless charge transport applications. Strain engineering on graphene has been achieved via random nanobubbles or artificial nanostructures on the substrate, but the highly localized and non-uniform pseudomagnetic fields can make spectroscopic probes of electronic structure difficult. Heterostructure engineering offers an alternative approach: By stacking graphene on top of another van der Waals material with large lattice mismatch at a desired twist angle, it is possible to generate large strain-induced pseudo magnetic fields uniformly over the entire heterostructure. Here, we report using nano-angle resolved photoemission spectroscopy (nano-ARPES) to probe the electronic bandstructure of a graphene/black phosphorus heterostructure (G/BP). By directly measuring the iso-energy contours of graphene and black phosphorus we determine a twist angle of 20-degrees in our heterostructure. High-resolution nano-ARPES of the graphene bands near the Fermi level reveals the emergence of flat bands located within the Dirac cone. The spacing of the flat bands is consistent with Landau level formation in graphene, and corresponds to a pseudo-field of 11.36 T. Our work provides a new way to study quantum Hall phases induced by strain in 2D materials and heterostructures.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源