论文标题
高级表征信息框架和定量见解,可照射的环形U-10ZR金属燃料
Advanced Characterization-Informed Framework and Quantitative Insight to Irradiated Annular U-10Zr Metallic Fuels
论文作者
论文摘要
基于U-10ZR的金属核燃料是下一代钠冷水反应堆的有前途的燃料候选者。爱达荷州国家实验室的研究经验可以追溯到1960年代。爱达荷州国家实验室研究人员在工程规模上积累了有关燃料性能的大量经验和知识。高级表征和缺乏适当的数据分析工具的局限性阻止了对燃料微观结构演化和辐射过程中特性退化的机械理解。本文提出了一个新的工作流程,再加上通过先进的辐照检查方法获得的域知识,以对裂变气泡和孔隙提供前所未有的量化见解,以及在高级测试反应器中辐照的环形燃料中的灯笼中的分布。在研究中,研究人员确定并确认存在具有ZR的二期相位,并产生沿热梯度的七个微观结构的定量比。此外,在定量比较了两个U-10ZR晚期燃料样品上裂变气泡的分布。获得了结论性发现,并允许根据两个晚期样品的大约67,000个裂变气泡来通过连接的气泡评估灯笼的运输。
U-10Zr-based metallic nuclear fuel is a promising fuel candidate for next-generation sodium-cooled fast reactors.The research experience of the Idaho National Laboratory for this type of fuel dates back to the 1960s. Idaho National Laboratory researchers have accumulated a considerable amount of experience and knowledge regarding fuel performance at the engineering scale. The limitation of advanced characterization and lack of proper data analysis tools prevented a mechanistic understanding of fuel microstructure evolution and properties degradation during irradiation. This paper proposed a new workflow, coupled with domain knowledge obtained by advanced post-irradiation examination methods, to provide unprecedented and quantified insights into the fission gas bubbles and pores, and lanthanide distribution in an annular fuel irradiated in the Advanced Test Reactor. In the study, researchers identify and confirm that the Zr-bearing secondary phases exist and generate the quantitative ratios of seven microstructures along the thermal gradient. Moreover, the distributions of fission gas bubbles on two samples of U-10Zr advanced fuels were quantitatively compared. Conclusive findings were obtained and allowed for evaluation of the lanthanide transportation through connected bubbles based on approximately 67,000 fission gas bubbles of the two advanced samples.