学术文献库

We report a detailed study of the magnetic, transport, and thermodynamic properties of Ce$_2$Te$_5$ single crystals, a layered $f$-electron van der Waals magnet. Four consecutive transitions at $\sim$ 5.2, 2.1, 0.9, and 0.4 K were observed in the $ac$-plane electrical resistivity $ρ$(T), which were further confirmed in specific heat $C_\textrm{p}$(T) measurements. Analysis of the magnetic susceptibility $χ$(T), the magnetic-field variation of $ρ$(T), and the increase of the first transition temperature ($T_\textrm{c} \sim$ 5.2 K) with applied magnetic field indicates ferromagnetic order, while the decrease of the other transitions with field suggests different states with dominant antiferromagnetic interactions below $T_2 \sim$ 2.1 K, $T_3 \sim$ 0.9 K, and $T_4$ = 0.4 K. Critical behavior analysis around $T_\textrm{c}$ that gives critical exponents $β= 0.31(2)$, $γ= 0.99(2)$, $δ= 4.46(1)$, $T_\textrm{c} = 5.32(1)$ K indicates that Ce$_2$Te$_5$ shows a three-dimensional magnetic critical behavior. Moreover, the Hall resistivity $ρ_{\textrm{xy}}$ indicates that Ce$_2$Te$_5$ is a multi-band system with a relatively high electron mobility $\sim 2900$ cm$^2$ V$^{-1}$ s$^{-1}$ near $T_\textrm{c}$, providing further opportunities for future device applications.