论文标题

laalo的离子调制$ _3 $/ktao $ _3 $界面的极端高动作二维电子气

Ionic modulation at the LaAlO$_3$/KTaO$_3$ interface for extreme high-mobility two-dimensional electron gas

论文作者

Yan, H., Zeng, S. W., Rubi, K., Omar, G. J., Zhang, Z. T., Goiran, M., Escoffier, W., Ariando, A.

论文摘要

由于许多新兴现象的共存,包括2D超导性和较大的Rashba旋转轨道耦合,基于5D过渡金属氧化物的二维电子系统(2DESS)已被视为现代电子学的潜在内部之一。然而,尽管电子质量较轻,但载体的迁移率是高性能设备的关键必需,但在5D氧化物设备中仍远远落后于其3D氧化物类似物。这些氧化物中的载体迁移率受到生长过程中产生的缺陷的不可避免的存在显着阻碍。在这里,我们报告了非常高的移动性($ \ sim $ 22650 cm $^2 $ v $^{ - 1} $ s $^{ - 1} $)的5D-2DE被限制在Laalo $ _3 $/ktao $ _3 $接口。 The high mobility, which is beyond the values observed in LaAlO$_3$/SrTiO$_3$ and $γ$-Al$_2$O$_3$/SrTiO$_3$ systems in the same carrier-density range, is achieved using the ionic-liquid gating at room temperature.我们假设离子液体门控会影响氧空位,并有效地减少界面处的任何障碍。我们透露,在各种后门电压中调查了密度和活动性,流动性遵循了power-law $μ\ propto n^{1.2} $,这表明离子 - 液体门控的Laalo $ _3 $/ktao $ _3 $ _3 $设备非常高质量,与我们的假设一致。此外,对在高磁场中测得的量子振荡的分析证实,高弹性电子占据了从TA中出现的电子子带:KTAO $ _3 $的5D轨道。

Due to the coexistence of many emergent phenomena, including 2D superconductivity and a large Rashba spin-orbit coupling, 5d transition metal oxides based two-dimensional electron systems (2DESs) have been prospected as one of the potential intrants for modern electronics. However, despite the lighter electron mass, the mobility of carriers, a key requisite for high-performance devices, in 5d-oxides devices remains far behind their 3d-oxides analogs. The carriers mobility in these oxides is significantly hampered by the inevitable presence of defects generated during the growth process. Here, we report very high mobility ($\sim$ 22650 cm$^2$V$^{-1}$s$^{-1}$) of 5d-2DES confined at the LaAlO$_3$/KTaO$_3$ interface. The high mobility, which is beyond the values observed in LaAlO$_3$/SrTiO$_3$ and $γ$-Al$_2$O$_3$/SrTiO$_3$ systems in the same carrier-density range, is achieved using the ionic-liquid gating at room temperature. We postulate that the ionic-liquid gating affects the oxygen vacancies and efficiently reduces any disorder at the interface. Investigating density and mobility in a broad range of back-gate voltage, we reveal that the mobility follows the power-law $μ\propto n^{1.2}$, indicating the very high quality of ionic-liquid-gated LaAlO$_3$/KTaO$_3$ devices, consistent with our postulate. Further, the analysis of the quantum oscillations measured in high magnetic fields confirms that the high-mobility electrons occupy the electronic sub-bands emerging from the Ta:5d orbitals of KTaO$_3$.

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