论文标题

相关系统高谐波产生的掺杂效应

Doping effects in high-harmonic generation from correlated systems

论文作者

Hansen, Thomas, Madsen, Lars Bojer

论文摘要

使用一维Hubbard模型,该模型通常用于描述,例如高$ T_C $超导蛋糕,我们从掺杂的,相关的材料中研究高谐波生成(HHG)。掺杂是通过从常规半填充情况中更改晶格中的电子数来建模的。对于相对较小的Hubbard $ U $,即小电子电子相关性,我们发现对动力学和HHG光谱的掺杂几乎没有影响。为了增加$ u $,掺杂程度对动态和光谱产生显着影响。我们通过基于准二粒的Doublon-Holon图片来解释这些发现。动力学分为两种类型,首先是Doublon和Holon运动,其次是Doublon-Holon对的创造和歼灭。掺杂会导致所有包含双龙或圆顶的配置。这些准粒子在能源上无需以无需额外的成本移动。这种运动无能为力增加了低谐波和中谐波的高谐波增益。我们讨论了在高$ $限制中,抗铁磁有序的不太可能随着掺杂率的增加而变得越来越不可能,并解释了相对于一半填充的情况,高阶谐波的相关下降。

Using the one-dimensional Hubbard model, which is commonly used for describing, e.g., high-$T_c$ superconducting cuprates, we study high-harmonic generation (HHG) from doped, correlated materials. Doping is modeled by changing the number of electrons in the lattice from the conventional half-filling case. For relatively small Hubbard $U$, i.e., small electron-electron correlation, we find little to no effect of doping on the dynamics and the HHG spectra. For increasing $U$ the degree of doping has a marked effect on the dynamics and spectra. We explain these findings through the quasiparticle-based doublon-holon picture. The dynamics are separated into two types, firstly doublon and holon movement, and, secondly, doublon-holon pair creation and annihilation. Doping results in all configurations containing doublons or holons. Those quasiparticles can move at no extra cost in energy regardless of the correlation level. This motion at no energy cost increases the high-harmonic gain for low and medium harmonic orders. We discuss that in the high-$U$ limit, antiferromagnetic ordering becomes increasingly unlikely with increasing doping rates and explain an associated drop in the high-order harmonics relative to the case of half filling.

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