论文标题

化学合成和材料发现

Chemical Synthesis and Materials Discovery

论文作者

Cheetham, Anthony K., Seshadri, Ram, Wudl, Fred

论文摘要

功能材料会影响我们生活的每个领域,从电子和计算设备到运输和健康。从这个角度来看,我们研究了综合发现与它们启用的科学突破之间的关系。通过追踪一些重要示例的发展,我们探讨了最初合成材料的方式和原因的原因以及如何随后认可其效用。确定了三种通用材料突破的途径。在少数情况下,例如铝硅酸盐沸石催化剂ZSM-5,通过使用基于早期工作的设计原理取得了重要的进步。偶然的突破性案例也很少见,例如Buckyball和Teflon(R)。然而,最常见的是,突破性重新利用了一种已经知道的化合物,通常是出于好奇或其他应用而制成的。通常,综合发现在数十年的发现之前的发现之前。主要例子包括用于锂离子电池的聚合物,拓扑绝缘子和电极。

Functional materials impact every area of our lives ranging from electronic and computing devices to transportation and health. In this Perspective, we examine the relationship between synthetic discoveries and the scientific breakthroughs that they have enabled. By tracing the development of some important examples, we explore how and why the materials were initially synthesized and how their utility was subsequently recognised. Three common pathways to materials breakthroughs are identified. In a small number of cases, such as the aluminosilicate zeolite catalyst ZSM-5, an important advance is made by using design principles based upon earlier work. There are also rare cases of breakthroughs that are serendipitous, such as the buckyball and Teflon(R). Most commonly, however, the breakthrough repurposes a compound that is already known and was often made out of curiosity or for a different application. Typically, the synthetic discovery precedes the discovery of functionality by many decades; key examples include conducting polymers, topological insulators and electrodes for lithium-ion batteries.

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