论文标题

带有三角形晶格的散装有机超导体中没有自旋敏感性降低

Absence of spin susceptibility decrease in a bulk organic superconductor with triangular lattice

论文作者

Saitou, Y., Ichikawa, N., Yamamoto, R., Kitamata, D., Suzuki, M., Yanagita, Y., Namaizawa, T., Komuro, S., Furukawa, T., Kato, R., Itou, T.

论文摘要

30多年来,对密切相关的电子系统中非S波非常规超导性的研究一直是凝聚态物理学的核心问题。在这种非常规的超导能力中,经常在各种准二维(Quasi-2d)散装系统中观察到D-Wave Cooper与反平行自旋配对。有趣的是,许多理论预测三角形晶格会导致D波配对不稳定,并可能导致更多异国情调的配对,例如平行自旋(旋转三曲线)配对。在这里,我们关注一个散装的有机三角晶格系统,在该系统中,超导性在非磁性莫特绝缘阶段附近。我们通过使用低功率核磁共振(NMR)测量来证明,超导状态的自旋敏感性在超导状态下保持正常状态。该结果表明该材料表现出自旋 - 三个超导性的可能性。我们的发现将带来洞察力,也将带有三角摩尔超级晶格的2D材料,这些材料也被认为在莫特般的绝缘状态附近也表现出非常规的超导性。

The study of non-s-wave unconventional superconductivities in strongly correlated-electron systems has been a central issue in condensed matter physics for more than 30 years. In such unconventional superconductivities, d-wave Cooper pairing with antiparallel spins has been often observed in various quasi-two-dimensional (quasi-2D) bulk systems. Interestingly, many theories predicted that the triangular lattice causes the d-wave pairing to be unstable and may lead to more exotic pairing such as parallel spin (spin-triplet) pairing. Here we focus on a bulk organic triangular-lattice system in which superconductivity emerges near a nonmagnetic Mott insulating phase. We demonstrate, by using low-power nuclear magnetic resonance (NMR) measurements, that the spin susceptibility of the superconducting state retains the normal state value even deep in the superconducting state. This result indicates the possibility that the material exhibits spin-triplet superconductivity. Our finding will bring insights also into understanding the 2D materials with triangular moire superlattices that are considered also to show unconventional superconductivities near Mott-like insulating states.

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