论文标题
观察裸露CRI3铁磁磁性中的内在晶相
Observation of intrinsic crystal phase in bare CrI3 ferromagnetism
论文作者
论文摘要
固有的结构阶段是基本物理特性的关键基础,也是创建具有前所未有的性能和独特功能的创新设备。 Van der Waals CRI3的远程铁磁顺序与层间堆叠顺序紧密绑定。但是,几层CRI3的内在结构仍然难以捉摸。在裸露的几层CRI3中尚未实验检测到的预测单斜相。在这里,我们发现了与层间抗铁磁耦合的几层CRI3的固有结构,在裸露和HBN已封闭的双层和三层式cri3中,在整个温度范围内,在裸露和HBN已封装的双层和三层式双层CRI3中都明确显示单斜均匀的堆叠范围。 HBN/CRI3/HBN异质结构,部分阻碍了CRI3的层间滑动。这项工作证明了几层CRI3的固有单斜晶晶相以及与磁性订单相关的相关性,从而为通过堆叠设计提供了许多创造磁纹理的机会。
Intrinsic structural phase is a crucial foundation for the fundamental physical properties, and for creating innovative devices with unprecedented performances and unique functionalities. Long-range ferromagnetic orders of van der Waals CrI3 are strongly tied with interlayer stacking orders. However, the intrinsic structure of few-layer CrI3 still remains elusive; the predicted monoclinic phase has not yet been experimentally detected in bare few-layer CrI3. Here we uncover the intrinsic structure of few-layer CrI3 with interlayer antiferromagnetic coupling, which unambiguously show monoclinic stacking in both bare and hBN-encapsulated bilayer and tri-five-layer CrI3 throughout an entire temperature range from 300 to 10 K. An exotic spring damping effect from hBN encapsulation layers is experimentally observed in hBN/CrI3/hBN heterostructures, which partly hinders interlayer sliding of CrI3. This work demonstrates the intrinsic monoclinic crystal phase of few-layer CrI3 and associated correlation with magnetic orders, opening up numerous opportunities for creating magnetic texture by stacking design.