论文标题

光合反应中心中的非马克维亚性:噪声诱导的量子相干透视

Non-Markovianity in photosynthetic reaction centers: A noise-induced quantum coherence perspective

论文作者

Wang, Zibo, Lim, Antonio V., Mirza, Imran M.

论文摘要

尽管在过去十年左右的时间里,尽管与炎热且嘈杂的环境相互作用,但在某些类型细菌和几乎各种植物中几乎完美光合产量的长期问题也几乎各种植物。通常,在这些解释中,光合反应中心被建模为五级量子热发动机,由于离散状态过渡与普通的马克维亚储层的耦合导致的Fano型干扰产生,负责增强光合效率的光合作用。在这项工作中,我们超越了早期作品中使用的born-markov近似值,并研究了具有洛伦兹光谱密度对轻型复合物动力学的非马克维亚环境的影响。

The long-standing problem of nearly perfect photosynthetic yield in some types of bacteria and nearly all kinds of plants despite the interaction with a hot and noisy environment has witnessed quantum optical explanations in the last decade or so. Typically in these explanations, photosynthetic reaction centers are modeled as five-level quantum heat engines where the generation of Fano-type interference due to the coupling of discrete state transitions with a common Markovian reservoir is held responsible for the enhancement of the photosynthetic efficiency. In this work, we go beyond the Born-Markov approximation used in the earlier works and study the impact of non-Markovian environments with Lorentzian spectral densities on the dynamics of light-harvesting complexes.

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