论文标题
原子定义技术的光学质量碳纳米管的确定性转移
Deterministic transfer of optical-quality carbon nanotubes for atomically defined technology
论文作者
论文摘要
当持续的设备缩放达到原子施加的最终极限时,基于原子上精确结构的技术将出现。然后,设备制造将需要具有确定的原子布置和组件组装而不会污染的构建块。在这里,我们报告了一种多功能的干燥转移技术,用于确定放置光学质量碳纳米管。单晶蒽被用作介质,通过轻度加热很容易升华,留下干净的纳米管,从而实现明亮的光致发光。我们能够在原位光学监测下以亚微米精度定位所需手性的纳米管,从而证明纳米管与光子晶体纳米氨腔的确定性耦合。还通过重复纳米管转移来设计和构建跨连接结构,该纳米管转移观察到Intertube激子转移。我们的结果代表了开发由原子精确组件和界面组成的设备开发的重要步骤。
When continued device scaling reaches the ultimate limit imposed by atoms, technology based on atomically precise structures is expected to emerge. Device fabrication will then require building blocks with identified atomic arrangements and assembly of the components without contamination. Here we report on a versatile dry transfer technique for deterministic placement of optical-quality carbon nanotubes. Single-crystalline anthracene is used as a medium which readily sublimes by mild heating, leaving behind clean nanotubes and thus enabling bright photoluminescence. We are able to position nanotubes of a desired chirality with a sub-micron accuracy under in-situ optical monitoring, thereby demonstrating deterministic coupling of a nanotube to a photonic crystal nanobeam cavity. A cross junction structure is also designed and constructed by repeating the nanotube transfer, where intertube exciton transfer is observed. Our results represent an important step towards development of devices consisting of atomically precise components and interfaces.