论文标题
位置控制的量子发射器,具有可再现的发射波长,氮化硼
Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
论文作者
论文摘要
低维分层材料中的单个光子发射器(SPE)最近由于吉祥的整合观点和该类别的材料提供的极端微型化的观点而引起了极大的兴趣。然而,量子发射器的空间位置和发射波长的准确控制本质上都是迄今为止缺乏的,因此阻碍了进一步的技术步骤,朝着可扩展的量子光子设备迈进。在这里,我们证明了高纯度合成六角硼(HBN)的SPE,可以通过所选位置的电子束激活。 SPE集合具有比立方发射波长更好的空间精度,从而为光学微结构中的集成开辟了道路。随后在可见范围内观察到稳定且明亮的单个光子发射,直到非共振激发激发后至室温。此外,低温发射波长是可重现的,宽度为3 meV的集合分布是一种统计分散,该分散体比在外部HBN样品中获得的最狭窄的波长差异低一个数量级。我们的发现构成了基于2D材料中相同的量子发射器来实现自上而下的集成设备的重要一步。
Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.