论文标题
高度可调的分层激子WS WS $ _2 $:线性量子限制的Stark效应与静电掺杂
Highly tunable layered exciton in bilayer WS$_2$: linear quantum confined Stark effect versus electrostatic doping
论文作者
论文摘要
在1H单层过渡金属二分裂基因中,倒置对称性被损坏,而反射对称性则保持不变。相反,在双层中,反转对称性恢复,但反射对称性被损坏。由于这些对称的对称性,在这里我们表明双层$ _2 $表现出与平面外电场线性线性的量子限制性恒定效应(QCSE),而与单层的二次效应相反。双层中独特的自由度与场驱动的部分相互转换之间的相互作用之间的相互作用产生了激子振荡器强度的巨大可调性。这使双层WS $ _2 $成为激子共振的原子较薄,可调的电吸附调制器的有前途的候选者,尤其是当堆叠在石墨烯层的顶部时,该层提供了一个超近似非辐射的放松通道。通过调整偏置构型,我们进一步表明,通过有效地将振荡器强度从中性到带电的激子传递,可以通过静电掺杂来很大程度上通过静电掺杂来调整激子响应。这些发现是针对高度可调,原子上的薄,紧凑和光的,在芯片上,可重新配置的下一代光电子的组件。
In 1H monolayer transition metal dichalcogenide, the inversion symmetry is broken, while the reflection symmetry is maintained. On the contrary, in the bilayer, the inversion symmetry is restored, but the reflection symmetry is broken. As a consequence of these contrasting symmetries, here we show that bilayer WS$_2$ exhibits a quantum confined Stark effect (QCSE) that is linear with the applied out-of-plane electric field, in contrary to a quadratic one for a monolayer. The interplay between the unique layer degree of freedom in the bilayer and the field driven partial inter-conversion between intra-layer and inter-layer excitons generates a giant tunability of the exciton oscillator strength. This makes bilayer WS$_2$ a promising candidate for an atomically thin, tunable electro-absorption modulator at the exciton resonance, particularly when stacked on top of a graphene layer that provides an ultra-fast non-radiative relaxation channel. By tweaking the biasing configuration, we further show that the excitonic response can be largely tuned through electrostatic doping, by efficiently transferring the oscillator strength from neutral to charged exciton. The findings are prospective towards highly tunable, atomically thin, compact and light, on chip, reconfigurable components for next generation optoelectronics.