论文标题

单层半导体中高度限制的平面内激子孔子

Highly Confined In-plane Exciton-Polaritons in Monolayer Semiconductors

论文作者

Epstein, Itai, Chaves, Andre J., Rhodes, Daniel A., Frank, Bettina, Watanabe, Kenji, Taniguchi, Takashi, Giessen, Harald, Hone, James C., Peres, Nuno M. R., Koppens, Frank H. L.

论文摘要

2D材料支持由材料激发和称为polariton的光子组成的准颗粒的独特激发。平面内传播极化子特别有趣,可以局限于单个单层并具有巨大的动量。在这项工作中,我们报告了一种在可见光频谱中支持单层过渡金属二基酮(TMD)支持的一种新型的面积繁殖偏光子,但尚未观察到。通过将电磁光场与单层TMD支持的激子的集体振荡偶联来描述这个2D面内激子孔子(2DEP)。我们暴露了激发2DEP所需的特定实验条件,并表明如果将TMD用六角形 - 硝酸盐(HBN)封装并冷却至低温温度,则可以创建这些条件。此外,我们将2DEPS的性质与相同光谱范围内的表面质量 - 叠正子(SPP)的性质进行比较,并发现2DEP在两个宽度的波长限制上表现出。最后,我们提出了两种配置,以实验2DEPS。

2D materials support unique excitations of quasi-particles that consist of a material excitation and photons called polaritons. Especially interesting are in-plane propagating polaritons which can be confined to a single monolayer and carry large momentum. In this work, we report the existence of a new type of in-plane propagating polariton, supported on monolayer transition-metal-dicalcogonide (TMD) in the visible spectrum, which has not yet been observed. This 2D in-plane exciton-polariton (2DEP) is described by the coupling of an electromagnetic light field with the collective oscillations of the excitons supported by monolayer TMDs. We expose the specific experimental conditions required for the excitation of the 2DEP and show that these can be created if the TMD is encapsulated with hexagonal-boron-nitride (hBN) and cooled to cryogenic temperatures. In addition, we compare the properties of the 2DEPs with those of surface-plasmons-polaritons (SPPs) at the same spectral range, and find that the 2DEP exhibit over two orders-of-magnitude larger wavelength confinement. Finally, we propose two configurations for the possible experimental observation of 2DEPs.

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