论文标题

在非极性物质中创建拓扑极性结构

Creating topological polar structure in a nonpolar matter

论文作者

Abid, Adeel Y., Sun, Yuanwei, Hou, Xu, Zhong, Xiangli, Tan, Congbing, Zhu, Ruixue, Chen, Haoyun, Qu, Ke, Li, Yuehui, Wu, Mei, Zhang, Jingmin, Wang, Jinbin, Liu, Kaihui, Bai, Xuedong, Yu, Dapeng, Wang, Jie, Li, Jiangyu, Gao, Peng

论文摘要

非平凡的拓扑结构在凝聚态物理学中提供了丰富的操场,包括流体动力学,超导性和铁磁学,它们承诺为后摩尔的纺纱和电子学提供替代的设备配置。实际上,磁性天空是为了进行高密度数据存储而积极追求的,而具有外来负电容的极性涡流可能会在微电子中实现超低功耗。在过去几十年中,对各种磁性纹理进行了广泛的研究,包括涡流,域壁和天空,近年来对极性拓扑的研究已经开始,从而发现了铁电材料中封闭结构域,涡旋和天空的发现。然而,拓扑极性结构的原子级创建主要局限于单个铁电系统,PBTIO3(PTO)具有较大的极化,对极性拓扑的一般性产生了怀疑,并限制了其潜在应用。在这项工作中,我们成功地创建了名义上非极性SRTIO3(STO)中的先前未实现的原子级极性抗vortices,扩大了拓扑结构的覆盖范围,并完成了极地拓扑中重要的缺失链接。这项工作对拓扑极性结构的形成有了广泛的新见解,并为寻找新的极性纹理提供了指导。

Nontrivial topological structures offer rich playground in condensed matter physics including fluid dynamics, superconductivity, and ferromagnetism, and they promise alternative device configurations for post-Moore spintronics and electronics. Indeed, magnetic skyrmions are actively pursued for high-density data storage, while polar vortices with exotic negative capacitance may enable ultralow power consumption in microelectronics. Following extensive investigations on a variety of magnetic textures including vortices, domain walls and skyrmions in the past decades, studies on polar topologies have taken off in recent years, resulting in discoveries of closure domains, vortices, and skyrmions in ferroelectric materials. Nevertheless, the atomic-scale creation of topological polar structures is largely confined in a single ferroelectric system, PbTiO3 (PTO) with large polarization, casting doubt on the generality of polar topologies and limiting their potential applications. In this work, we successfully create previously unrealized atomic-scale polar antivortices in the nominally nonpolar SrTiO3 (STO), expanding the reaches of topological structures and completing an important missing link in polar topologies. The work shed considerable new insight into the formation of topological polar structures, and offers guidance in searching for new polar textures.

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