论文标题

抗铁磁化合物EUCU2GE2的独特电子状态的价值转变的量子关键性

Quantum Criticality of Valence Transition for the Unique Electronic State of Antiferromagnetic Compound EuCu2Ge2

论文作者

Gouchi, Jun, Miyake, Kazumasa, Iha, Wataru, Hedo, Masato, Nakama, Takao, Onuki, Yoshichika, Uwatoko, Yoshiya

论文摘要

通过最高10 GPA的电阻率测量值,压力对抗铁磁(AF)化合物EUCU2GE2的独特电子状态的影响已在10 mk至300​​ K的宽范围内测量。在环境压力下Tn = 15 K的neEL温度随着压力的增加而单调地增加,并在6.2 GPa时变为Tn = 27 K,但在PC = 6.5 GPA时突然下降至零,降至零,这表明欧盟的量子临界点(QCP)从几乎分裂的状态到具有数量的重量。基于rhomag的费米液体关系= rhomag0 + at^2的rhomag0和从低温电阻率获得的值和PC周围的尖锐峰值。从功率定律依赖性rhomag = rhomag0 + bt^n获得的指数n显然小于p = pc =6。5gpa的1.5,这是在AF-QCP上预期的。这些结果表明,PC与PV一致,对应于价转换压力PV的量子临界。根据广义的Kadowaki-Woods关系估算的电子特异性热系数在PC周围约为510 MJ/mol K^2,这表明形成了一个重毛状状态。

The effect of pressure on the unique electronic state of the antiferromagnetic (AF) compound EuCu2Ge2 has been measured in a wide temperature range from 10 mK to 300 K by electrical resistivity measurements up to 10 GPa. The Neel temperature of TN = 15 K at ambient pressure increases monotonically with increasing pressure and becomes a maximum of TN = 27 K at 6.2 GPa but suddenly drops to zero at Pc = 6.5 GPa, suggesting the quantum critical point (QCP) of the valence transition of Eu from a nearly divalent state to that with trivalent weight. The rhomag0 and A values obtained from the low-temperature electrical resistivity based on the Fermi liquid relation of rhomag = rhomag0 + AT^2 exhibit huge and sharp peaks around Pc. The exponent n obtained from the power law dependence rhomag = rhomag0 + BT^n is clearly less than 1.5 at P = Pc = 6. 5 GPa, which is expected at the AF-QCP. These results indicate that Pc coincides with Pv, corresponding to the quantum criticality of the valence transition pressure Pv. The electronic specific heat coefficient, estimated from the generalized Kadowaki-Woods relation, is about 510 mJ/mol K^2 around Pc, suggesting the formation of a heavy-fermion state.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源