论文标题

来自驱动的光子声子的可调剪切应变

Tunable shear strain from resonantly driven optical phonons

论文作者

Hortensius, J. R., Afanasiev, D., Sasani, A., Bousquet, E., Caviglia, A. D.

论文摘要

应变工程最近已扩展到Ultrafast时标,驱动金属压形器相变和超声波消灭阵线的传播。然而,尚未解决非线性晶格动力学基础的基础界面光电相切换。在这里,我们关注的是通过冲动的谐振激发Laalo $ _3 $单晶引发的晶格动力学,这是氧化物电子产品最广泛使用的基板之一。我们表明,离子拉曼散射驱动驱动相干的氧气八面体围绕高对称性晶体轴旋转,我们通过DFT计算确定了基础的声子 - phonon耦合通道。谐振晶格激发显示可产生纵向和横向声波包,这些波袋由各向异性光学诱导的菌株进出平衡。重要的是,发现剪切应变波袋是在声子共振下以非凡效率产生的,与更传统的纵向声波相当,为超快材料控制打开了令人兴奋的观点。

Strain engineering has been extended recently to the ultrafast timescales, driving metal-insulator phase transitions and the propagation of ultrasonic demagnetization fronts. However, the non-linear lattice dynamics underpinning interfacial optoelectronic phase switching have not yet been addressed. Here we focus on the lattice dynamics initiated by impulsive resonant excitation of polar lattice vibrations in LaAlO$_3$ single crystals, one of the most widely utilized substrates for oxide electronics. We show that ionic Raman scattering drives coherent oxygen octahedra rotations around a high-symmetry crystal axis and we identify, by means of DFT calculations, the underlying phonon-phonon coupling channel. Resonant lattice excitation is shown to generate longitudinal and transverse acoustic wavepackets, enabled by anisotropic optically-induced strain in and out of equilibrium. Importantly, shear strain wavepackets are found to be generated with extraordinary efficiency at the phonon resonance, being comparable in amplitude to the more conventional longitudinal acoustic waves, opening exciting perspectives for ultrafast material control.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源