论文标题
半谷金属和量子异常山谷效果的概念
Concept of the half-valley-metal and quantum anomalous valley Hall effect
论文作者
论文摘要
山谷是动量空间的电子带结构中的能量极值,除了电荷和自旋外,还被认为是一种新的电子自由度。现在,这些研究集中在山谷的自由度上,现在构成了凝聚态物理学的新兴领域,即valleytronics,其发展正是遵循旋转型的旋转型自由度的发展。在这里,类似于一个自旋通道中的旋转三位型的半米,而另一种是绝缘的,我们提出了半谷化 - 金属的概念,其中传导电子本质上是100%山谷极化的,即使考虑了自旋旋转的旋转相互作用。将第一原理的计算与两波段KP模型相结合,形成半谷金属的物理机制被照亮了。以强大交换相互作用为例的Ferrovalley H-Fecl2单层单层,我们发现强的电子相关效应可以诱导Ferrovalley诱导半谷利金属转变。由于依赖山谷的光学选择规则,这种系统可以透明地与左旋极化的光透明,但是将反映右圆形光线,这又可以用作检测半瓦利 - 金属状态的关键方法。此外,我们发现在SO获得的半谷金属状态下,传导谷表现出狄拉克锥样线性能量分散体。有趣的是,随着相关效应的增加,系统再次逐渐遵循相同的光学选择规则。我们确认,在这种特定情况下,由单个自旋组成的价带具有非零的Chern数,因此出现了固有的量子异常山谷大厅效应。我们的发现为ValleyTronics的功能2D材料设计开辟了一条吸引人的途径。
Valley, the energy extrema in the electronic band structure at momentum space, is regarded as a new degree of freedom of electrons, in addition to charge and spin. The studies focused on valley degree of freedom now form an emerging field of condensed matter physics, i.e. valleytronics, whose development is exactly following that of spintronics which focuses on the spin degree of freedom. Here, in analogy to half-metals in spintronics with one spin channel is conducting whereas the other is insulating, we propose the concept of half-valley-metal, in which conduction electrons are intrinsically 100% valley polarized, as well as 100% spin-polarized even when spin-orbit interactions are considered. Combining first-principles calculations with two-band kp model, the physical mechanism to form the half-valley-metal is illuminated. Taking the ferrovalley H-FeCl2 monolayer with strong exchange interaction as an example, we find that the strong electron correlation effect can induce the ferrovalley to half-valley-metal transition. Due to the valley-dependent optical selection rules, such system could be transparent to, e.g., left-circularly polarized light, yet the right-circularly polarized light will be reflected, which can in turn be used as a crucial method to detect half-valley-metal state. In addition, we find that in the so obtained half-valley-metal state, the conduction valley demonstrates Dirac cone-like linear energy dispersion. Interestingly, with the increase of the correlation effect, the system becomes insulating again with all valleys follow same optical selection rule. We confirm that in this specific case, the valence bands, which consist of single spin, possess non-zero Chern number and consequently intrinsic quantum anomalous valley Hall effect emerges. Our findings open an appealing route toward functional 2D materials design of valleytronics.