论文标题

不足的$ \ text {hgba} _2 \ text {cuo} _ {4+δ} $由中子散射调查

Phonon spectrum of underdoped $\text{HgBa}_2\text{CuO}_{4+δ}$ investigated by neutron scattering

论文作者

Ahmadova, I., Sterling, T. C., Sokolik, A. C., Abernathy, D. L., Greven, M., Reznik, D.

论文摘要

库酸盐表现出沿[100],即Cu-O键方向的波形显着的电荷密度波(CDW)不稳定性。尽管CDW顺序在中等掺杂和低温下最突出,但越来越多的证据证明了整个温度掺杂相图的动态电荷相关性。特别是,已经观察到起步电荷顺序的特征是声子软化和/或在CDW波形附近大约一半穿过Brillouin区域。这项工作的大部分都集中在中等掺杂的铜岩上,CDW顺序是可靠的,或最佳的样本,超导过渡温度($ T_C $)最大。在这里,我们提出了简单四边形$ \ text {hgba} _2 \ text {cuo} _ {4+δ} $($ t_c = 55 $ k)的飞行时间中子散射研究,在先前的工作中显示CDW订单很弱。我们采用并展示了一种基于软件的新技术,该技术为有用的数据挖掘了大量测量的布里渊区,以提高准确性和计数统计信息。密度功能理论尚未提供$ \ text {hgba} _2 \ text {cuo} _ {4+δ} $中的声子的准确描述,但是我们找到了正确的参数集来合理地重现数据。值得注意的例外是沿[100]的纵向Cu-O键拉伸分支中的分散剂。这种差异表明,尽管CDW顺序较弱,但在低掺杂的光子声子范围内存在显着的动态电荷相关性,靠近超导穹顶的边缘。

The cuprates exhibit a prominent charge-density-wave (CDW) instability with wavevector along [100], i.e., the Cu-O bond direction. Whereas CDW order is most prominent at moderate doping and low temperature, there exists increasing evidence for dynamic charge correlations throughout a large portion of the temperature-doping phase diagram. In particular, signatures of incipient charge order have been observed as phonon softening and/or broadening near the CDW wavevector approximately half-way through the Brillouin zone. Most of this work has focused on moderately-doped cuprates, for which the CDW order is robust, or on optimally-doped samples, for which the superconducting transition temperature ($T_c$) attains its maximum. Here we present a time-of-flight neutron scattering study of phonons in simple-tetragonal $\text{HgBa}_2\text{CuO}_{4+δ}$ ($T_c = 55$ K) at a low doping level where prior work showed the CDW order to be weak. We employ and showcase a new software-based technique that mines the large number of measured Brillouin zones for useful data in order to improve accuracy and counting statistics. Density-functional theory has not provided an accurate description of phonons in $\text{HgBa}_2\text{CuO}_{4+δ}$, yet we find the right set of parameters to qualitatively reproduce the data. The notable exception is a dispersion minimum in the longitudinal Cu-O bond-stretching branch along [100]. This discrepancy suggests that, while CDW order is weak, there exist significant dynamic charge correlations in the optic phonon range at low doping, near the edge of the superconducting dome.

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